Effect of defect density and energy level mismatch on the performance of perovskite solar cells by numerical simulation

Computer simulation; Defect density; Lead compounds; Nickel oxide; Numerical models; Perovskite; Solar cells; Defect energy level; Defect levels; Hole transport materials; Interfacial defect; Organic-inorganic; Perovskite layers; Power conversion efficiencies; SCAPS-1D; Perovskite solar cells

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Main Authors: Jamal M.S., Shahahmadi S.A., Chelvanathan P., Asim N., Misran H., Hossain M.I., Amin N., Sopian K., Akhtaruzzaman M.
Other Authors: 55887499100
Format: Article
Published: Elsevier GmbH 2023
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spelling my.uniten.dspace-247262023-05-29T15:26:18Z Effect of defect density and energy level mismatch on the performance of perovskite solar cells by numerical simulation Jamal M.S. Shahahmadi S.A. Chelvanathan P. Asim N. Misran H. Hossain M.I. Amin N. Sopian K. Akhtaruzzaman M. 55887499100 55567116600 35766323200 55902096700 6506899840 36448414000 7102424614 7003375391 57195441001 Computer simulation; Defect density; Lead compounds; Nickel oxide; Numerical models; Perovskite; Solar cells; Defect energy level; Defect levels; Hole transport materials; Interfacial defect; Organic-inorganic; Perovskite layers; Power conversion efficiencies; SCAPS-1D; Perovskite solar cells The defects at the absorber and interface layer of organic-inorganic lead halide perovskite solar cells are unfavorable for efficiency as well as the stability. In this study, we have performed the numerical simulation on inverted planar structure perovskite solar cell based on NiO as a hole transport material (HTM) by SCAPS -1 D. Here we investigated the effects of defect density and energy level of the perovskite absorber layer and perovskite/HTM interface layer on the performance, respectively. The analysis revealed that values of J sc , V oc , and FF of perovskite solar cells are significantly reduced with increasing the defect density of perovskite layer. The power conversion efficiency severely reduced from 25 to 5% when the defect density increased from 10 13 to 10 18 cm ?3 , respectively. A similar trend was also found in case of interfacial defect between Perovskite and HTM layer. It was found that the defect energy level more than 0.3 eV above conduction band of perovskite has almost no detrimental effect on the device's efficiency. � 2019 Elsevier GmbH Final 2023-05-29T07:26:17Z 2023-05-29T07:26:17Z 2019 Article 10.1016/j.ijleo.2018.12.163 2-s2.0-85063291071 https://www.scopus.com/inward/record.uri?eid=2-s2.0-85063291071&doi=10.1016%2fj.ijleo.2018.12.163&partnerID=40&md5=f23f4f3dfb8d18ac8cabb225bad713ba https://irepository.uniten.edu.my/handle/123456789/24726 182 1204 1210 Elsevier GmbH Scopus
institution Universiti Tenaga Nasional
building UNITEN Library
collection Institutional Repository
continent Asia
country Malaysia
content_provider Universiti Tenaga Nasional
content_source UNITEN Institutional Repository
url_provider http://dspace.uniten.edu.my/
description Computer simulation; Defect density; Lead compounds; Nickel oxide; Numerical models; Perovskite; Solar cells; Defect energy level; Defect levels; Hole transport materials; Interfacial defect; Organic-inorganic; Perovskite layers; Power conversion efficiencies; SCAPS-1D; Perovskite solar cells
author2 55887499100
author_facet 55887499100
Jamal M.S.
Shahahmadi S.A.
Chelvanathan P.
Asim N.
Misran H.
Hossain M.I.
Amin N.
Sopian K.
Akhtaruzzaman M.
format Article
author Jamal M.S.
Shahahmadi S.A.
Chelvanathan P.
Asim N.
Misran H.
Hossain M.I.
Amin N.
Sopian K.
Akhtaruzzaman M.
spellingShingle Jamal M.S.
Shahahmadi S.A.
Chelvanathan P.
Asim N.
Misran H.
Hossain M.I.
Amin N.
Sopian K.
Akhtaruzzaman M.
Effect of defect density and energy level mismatch on the performance of perovskite solar cells by numerical simulation
author_sort Jamal M.S.
title Effect of defect density and energy level mismatch on the performance of perovskite solar cells by numerical simulation
title_short Effect of defect density and energy level mismatch on the performance of perovskite solar cells by numerical simulation
title_full Effect of defect density and energy level mismatch on the performance of perovskite solar cells by numerical simulation
title_fullStr Effect of defect density and energy level mismatch on the performance of perovskite solar cells by numerical simulation
title_full_unstemmed Effect of defect density and energy level mismatch on the performance of perovskite solar cells by numerical simulation
title_sort effect of defect density and energy level mismatch on the performance of perovskite solar cells by numerical simulation
publisher Elsevier GmbH
publishDate 2023
_version_ 1806428362887921664
score 13.214268