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Linear and nonlinear optical susceptibilities and the hyperpolarizability of borate LiBaB9O15 single-crystal: theory and experiment

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Main Authors: Ali Hussain, Reshak, Prof. Dr., Chen, Xuean, Auluck, Sushil, Kamarudin, Hussin, Brig. Jen. Dato' Prof. Dr., Chysky, Jan, Wojciechowski, Artur, Kityk, Ivan V.
Other Authors: maalidph@yahoo.co.uk
Format: Article
Language:English
Published: American Chemical Society 2014
Subjects:
Hyper-polarizability
Linear optical properties
Nonlinear optical susceptibilities
Second-order nonlinear optical
Single crystal x-ray diffraction
Online Access:http://dspace.unimap.edu.my:80/dspace/handle/123456789/35400
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spelling my.unimap-354002017-11-29T09:10:42Z Linear and nonlinear optical susceptibilities and the hyperpolarizability of borate LiBaB9O15 single-crystal: theory and experiment Ali Hussain, Reshak, Prof. Dr. Chen, Xuean Auluck, Sushil Kamarudin, Hussin, Brig. Jen. Dato' Prof. Dr. Chysky, Jan Wojciechowski, Artur Kityk, Ivan V. maalidph@yahoo.co.uk sauluck@gmail.com kamarudin@unimap.edu.my jan.Chysky@fs.cvut.cz awojciech2013@wp.pl ikityk@el.pcz.czest.pl Hyper-polarizability Linear optical properties Nonlinear optical susceptibilities Second-order nonlinear optical Single crystal x-ray diffraction Link to publisher's homepage at http://pubs.acs.org/ The single-crystal borate LiBaB9O15 was synthesized by a high-temperature solution reaction and structurally determined by the single-crystal X-ray diffraction technique. It crystallizes in the noncentrosymmetric space group R3c and features a three-dimensional ∞ 3[B9O15]3- anionic framework, with infinite channels in which the Li+ and Ba 2+ cations are located. The linear optical properties were investigated experimentally in terms of the absorption spectrum, which reveals an optical gap of 5.17 eV. In addition we have calculated the linear optical properties using state-of-the-art all-electron full potential linearized augmented plane wave method. The nonlinear optical susceptibilities, namely, the second harmonic generation and the hyperpolarizability of the single-crystal borate LiBaB9O15 are calculated and evaluated at a static limit and at λ = 1064 nm. The calculation shows there exists three second-order nonlinear optical susceptiblities tensors components. We present measurements of the IR spectra in the range 500-2000 cm-1, and the second harmonic generation was performed using a Quantel 15 ns Nd:YAG laser operating at 1064 nm. 2014-06-11T14:46:48Z 2014-06-11T14:46:48Z 2013-11 Article Journal of Physical Chemistry B, vol. 117(45), 2013, pages 14141-14150 1520-6106 (Print) 1520-5207 (Online) http://pubs.acs.org/doi/abs/10.1021/jp4077905 http://dspace.unimap.edu.my:80/dspace/handle/123456789/35400 10.1021/jp4077905 en American Chemical Society
institution Universiti Malaysia Perlis
building UniMAP Library
collection Institutional Repository
continent Asia
country Malaysia
content_provider Universiti Malaysia Perlis
content_source UniMAP Library Digital Repository
url_provider http://dspace.unimap.edu.my/
language English
topic Hyper-polarizability
Linear optical properties
Nonlinear optical susceptibilities
Second-order nonlinear optical
Single crystal x-ray diffraction
spellingShingle Hyper-polarizability
Linear optical properties
Nonlinear optical susceptibilities
Second-order nonlinear optical
Single crystal x-ray diffraction
Ali Hussain, Reshak, Prof. Dr.
Chen, Xuean
Auluck, Sushil
Kamarudin, Hussin, Brig. Jen. Dato' Prof. Dr.
Chysky, Jan
Wojciechowski, Artur
Kityk, Ivan V.
Linear and nonlinear optical susceptibilities and the hyperpolarizability of borate LiBaB9O15 single-crystal: theory and experiment
description Link to publisher's homepage at http://pubs.acs.org/
author2 maalidph@yahoo.co.uk
author_facet maalidph@yahoo.co.uk
Ali Hussain, Reshak, Prof. Dr.
Chen, Xuean
Auluck, Sushil
Kamarudin, Hussin, Brig. Jen. Dato' Prof. Dr.
Chysky, Jan
Wojciechowski, Artur
Kityk, Ivan V.
format Article
author Ali Hussain, Reshak, Prof. Dr.
Chen, Xuean
Auluck, Sushil
Kamarudin, Hussin, Brig. Jen. Dato' Prof. Dr.
Chysky, Jan
Wojciechowski, Artur
Kityk, Ivan V.
author_sort Ali Hussain, Reshak, Prof. Dr.
title Linear and nonlinear optical susceptibilities and the hyperpolarizability of borate LiBaB9O15 single-crystal: theory and experiment
title_short Linear and nonlinear optical susceptibilities and the hyperpolarizability of borate LiBaB9O15 single-crystal: theory and experiment
title_full Linear and nonlinear optical susceptibilities and the hyperpolarizability of borate LiBaB9O15 single-crystal: theory and experiment
title_fullStr Linear and nonlinear optical susceptibilities and the hyperpolarizability of borate LiBaB9O15 single-crystal: theory and experiment
title_full_unstemmed Linear and nonlinear optical susceptibilities and the hyperpolarizability of borate LiBaB9O15 single-crystal: theory and experiment
title_sort linear and nonlinear optical susceptibilities and the hyperpolarizability of borate libab9o15 single-crystal: theory and experiment
publisher American Chemical Society
publishDate 2014
url http://dspace.unimap.edu.my:80/dspace/handle/123456789/35400
_version_ 1643802758915031040
score 13.222552

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